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排序方式: 共有175条查询结果,搜索用时 140 毫秒
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ThebufferingeffectsofaquaticsedimentsagainstacidicdepositionLiaoBohan;TangHongxiao(ResearehCenterforEco-EnvironmentalSciences... 相似文献
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有机蒙脱石负载纳米铁去除溶液中四溴双酚A的研究 总被引:4,自引:2,他引:2
研究了改性蒙脱石负载纳米铁材料(NZVI-CMT)在甲醇-水体系中对四溴双酚A(TBBPA)的去除作用,并确定了反应温度、TBBPA初始浓度以及材料投加量等因素对去除效果的影响.结果表明,在25℃条件下,0.02 g NZVI-CMT对初始浓度为10 mg·L-1TBBPA溶液的去除率可达97.5%,而且NZVI-CMT对TBBPA的去除率明显高于两种单一材料即纳米零价铁(NZVI)及有机蒙脱石(CMT)的去除率(18.3%、67.3%),同时也大于两者之和(85.6%).利用NZVI-CMT对TBBPA进行重复去除实验时,前3次的去除率均可达到90%以上.通过检测降解产物并分析材料对TBBPA去除过程的特性,发现NZVI-CMT对TBBPA的去除以吸附为主,并伴有少量还原脱溴反应发生,而且较高的反应温度对降解反应有利. 相似文献
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Yilei Yu Xianfang Song Yinghua Zhang Fandong Zheng Ji Liang Dongmei Han Ying M Hongmei Bu 《环境科学学报(英文版)》2013,25(9):1754-1763
Reclaimed water was successfully used to recover the dry Chaobai River in Northern China, but groundwater may be polluted. To ensure groundwater protection, it is therefore critical to identify the governing factors of groundwater chemistry. Samples of reclaimed water, river and groundwater were collected monthly at Chaobai River from January to September in 2010. Fifteen water parameters were analyzed. Two kinds of reclaimed water were different in type (Na-Ca-Mg-Cl-HCO3 or Na-Ca-Cl-HCO3 ) and concentration of nitrogen. The ionic concentration and type in river were similar to reclaimed water. Some shallow wells near the river bed had the same type (Na-Ca-Mg-Cl-HCO3 ) and high concentration as reclaimed water, but others were consistent with the deep wells (Ca-Mg-HCO3 ). Using cluster analysis, the 9 months were divided into two periods (dry and wet seasons), and all samples were grouped into several spatial clusters, indicating different controlling mechanisms. Principal component analysis and conventional ionic plots showed that calcium, magnesium and bicarbonate were controlled by water-rock interaction in all deep and some shallow wells. This included the dissolution of calcite and carbonate weathering. Sodium, potassium, chloride and sulfate in river and some shallow wells recharged by river were governed by evaporation crystallization and mixing of reclaimed water. But groundwater chemistry was not controlled by precipitation. During the infiltration of reclaimed water, cation exchange took place between (sodium, potassium) and (calcium, magnesium). Nitrification and denitrification both happened in most shallow groundwater, but only denitrification in deep groundwater. 相似文献
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聚合铝铁对A2/O系统 EPS及生物絮凝性能的影响 总被引:1,自引:0,他引:1
通过向实验室构建的A2/O模型好氧池末端投加聚合铝铁(PAFC)来强化系统的生物除磷,使得出水总磷达到《城市污水处理厂污染物排放标准GB 18918-2002》中的一级A标准,并重点分析投加的PAFC对A2/O系统中活性污泥胞外聚合物(EPS)和活性污泥生物絮凝性能的影响.结果表明,随着PAFC投药量的增加,A2/O系统活性污泥EPS总量变化不大,但EPS组分中蛋白/多糖含量的比值逐渐降低,由投药前的3.30降低至投药后的2.30;EPS中金属离子含量逐渐增加,在厌氧-缺氧-好氧的运行周期内,各处理单元污泥的EPS中金属铝离子含量增加.投加PAFC后,活性污泥颗粒变大,二沉池出水的Zeta电位明显降低,由投药前-15.83 mV降低至-21.20 mV,污泥产量增加.因此,适量投加PAFC后,生物絮凝性能得到改善,出水中悬浊颗粒减少,出水水质变好. 相似文献
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M. W. Kress R. Baker S. J. Ursic 《Journal of the American Water Resources Association》1990,26(5):747-756
ABSTRACT: The deposition and chemistry of precipitation were estimated for one year in two forest ecosystems in the South-Central United States. Precipitation, throughfall, litter leachate, and soil leachate were analyzed for a small catchment of pine-hardwoods in southeastern Oklahoma and for a catchment of loblolly pines (Pinus taeda L.) in northern Mississippi. In the pine-hardwood forest, 98 percent of the acid deposition was neutralized, 50 percent in the forest canopy, and 48 percent in the forest floor. In the pine forest, 75 percent of the acid deposition was neutralized, all in the forest floor. The pine-hardwood ecosystem accumulated sulfate, nitrate, and ammonia ions, and lost base cations. During seasons of deficient precipitation, dry deposition appeared to enrich the concentrations of hydrogen, nitrate, sulfate, and ammonia ions in throughfall samples at both locations. 相似文献
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Wendy A. Rice Steven M. Gorelick 《Journal of the American Water Resources Association》1985,21(6):919-930
A graphical inverse method for determining the regional transmissivity distribution was applied to three field problems. The study areas were the Hanford Site, Washington; the Rocky Mountain Arsenal, Colorado; and the Nevada Test Site, Nevada. This method can aid in flow system conceptualization by revealing the location of bedrock controls for groundwater flow. It is a valuable tool for aiding the hydrogeologist in asking questions about the nature of trends in the pattern of transmissivity values. Quantitative estimates of regional transmissivities can be used as starting points for further parameter refinement. Sensitivity analysis using Monte Carlo simulation shows that quantitative estimates of transmissivity can be obtained when measurement error in the hydraulic head does not cause a large error in the hydraulic gradient. 相似文献
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Mary Beth Adams James N. Kochenderfer Pamela J. Edwards 《Water, Air, & Soil Pollution: Focus》2007,7(1-3):267-273
In 1989, a watershed acidification experiment was begun on the Fernow Experimental Forest in West Virginia, USA. Ammonium
sulfate fertilizer (35.5 kg N ha−1 yr−1and 40.5 kg S ha−1 yr−1) was applied to a forested watershed (WS3) that supported a 20-year-old stand of eastern deciduous hardwoods. Additions of
N and S are approximately twice the ambient deposition of nitrogen and sulfur in the adjacent mature forested watershed (WS4),
that serves as the reference watershed for this study. Acidification of stream water and soil solution was documented, although
the response was delayed, and acidification processes appeared to be driven by nitrate rather than sulfate. As a result of
the acidification treatment, nitrate solution concentrations increased below all soil layers, whereas sulfate was retained
by all soil layers after only a few years of the fertilization treatments, perhaps due to adsorption induced from decreasing
sulfate deposition. Based on soil solution monitoring, depletion of calcium and magnesium was observed, first from the upper
soil horizons and later from the lower soil horizons. Increased base cation concentrations in stream water also were documented
and linked closely with high solution levels of nitrate. Significant changes in soil chemical properties were not detected
after 12 years of treatment, however. 相似文献
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